Volume 8 Issue 2
May  2023
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Article Navigation >  Journal of Bioresources and Bioproducts  > 2023  >  8(2): 136-145
Zhangkang Li, Jamie LeBlanc, Hitendra Kumar, Hongguang Zhang, Weijun Yang, Xiao He, Qingye Lu, Jeffrey Van Humbeck, Keekyoung Kim, Jinguang Hu. Super-anti-freezing, tough and adhesive titanium carbide and L-ornithine-enhanced hydrogels[J]. Journal of Bioresources and Bioproducts, 2023, 8(2): 136-145. doi: 10.1016/j.jobab.2023.01.005
Citation: Zhangkang Li, Jamie LeBlanc, Hitendra Kumar, Hongguang Zhang, Weijun Yang, Xiao He, Qingye Lu, Jeffrey Van Humbeck, Keekyoung Kim, Jinguang Hu. Super-anti-freezing, tough and adhesive titanium carbide and L-ornithine-enhanced hydrogels[J]. Journal of Bioresources and Bioproducts, 2023, 8(2): 136-145. doi: 10.1016/j.jobab.2023.01.005
shu

Super-anti-freezing, tough and adhesive titanium carbide and L-ornithine-enhanced hydrogels

doi: 10.1016/j.jobab.2023.01.005
  • a.

    Department of Biomedical Engineering, University of Calgary, Calgary, University Drive NW, Calgary, AB T2N 1N4, Canada

  • b.

    Department of Chemistry, University of Calgary, University Drive NW, Calgary T2N 1N4, Alberta, Canada

  • c.

    Department of Mechanical and Manufacturing Engineering, University of Calgary, University Drive NW, Calgary T2N 1N4, Alberta, Canada

  • d.

    Pathology and Laboratory Medicine, Cumming School of Engineering, University of Calgary, Hospital Drive NW, T2N 4N1, Alberta, Canada

  • e.

    Department of Chemical and Petroleum Engineering, University of Calgary, University Drive NW, Calgary T2N 1N4, Alberta, Canada

  • f.

    Key Laboratory of Synthetic and Biological Colloids, Ministry of Education, School of Chemical and Material Engineering, Jiangnan University, Wuxi, Jiangsu, 214122, China

More Information
    Abstract
  • Hydrogels are highly porous three-dimensional crosslinked polymer networks consisting of hydrophilic polymers, employed most practically in medicine and industry, often as biosensors. Simple hydrogels suffer limitations in their mechanical properties, such as tensile and compression, and freeze at sub-zero temperatures, which compromise their ability as useful biosensors. In this study, the incorporation of L-ornithine-based zwitterionic monomer (OZM), titanium carbide (MXene), and glycerol within polyacrylamide hydrogels was used to prepare a novel polyacrylamide/polyL-ornithine-based zwitterion/MXene (PAM/Porn/MXene) hydrogel to improve the mechanical, adhesion, and anti-freezing properties of pure polyacrylamide hydrogels. This study also analyzed the mechanical strength (tensile and compression), adhesion, and anti-freezing properties of a novel PAM/Porn/MXene hydrogel at 1%, 4%, and 10% MXene concentrations to establish to what extent the conductive MXene material enhanced these properties and concluded that the tensile and compressive properties improved linearly with the increase in the concentrations of MXene, adhesion decreased with the increased MXene concentrations, and synergistic interaction between MXene and OZM significantly improved the anti-freezing properties up to –80 ℃.

     

    • Declaration of Competing Interest  There are no conflicts to declare.
    Supplementary material associated with this article can be found, in the online version, at doi:10.1016/j.jobab.2023.01.005.
    Supplementary materials
    1 These authors contributed equally to this work.
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